Inelastic neutron scattering study of the magnetic field dependence of the quantum dipolar garnet
Phys. Rev. B 111, 214419 – Published 10 June, 2025
DOI: https://doi.org/10.1103/r5md-t5z7
Abstract
The garnet compound is a fascinating material that is considered highly suitable for low-temperature refrigeration, via the magnetocaloric effect, in addition to enabling the exploration of quantum states with long-range dipolar interactions. It has previously been theorized that the magnetocaloric effect can be enhanced in via magnetic soft mode excitations, which in the hyperkagome structure would be derived from an emergent magnetic structure formed from nanosized ten-spin loops. We study the magnetic field dependence of bands of magnetic soft mode excitations in the effective spin hyperkagome compound using single-crystal inelastic neutron scattering. We probe the magnetically short-ranged ordered state, in which we determine magnetic nanoscale structures coexisting with a fluctuating state, and the magnetically saturated state, from which we determine the relevant magnetic interactions. We determine that can be described as a quantum dipolar magnet with perturbative weak near-neighbor and interhyperkagome exchange interaction. The magnetic excitations, under the application of a magnetic field, reveal highly robust soft modes with distinctive signatures of the quantum nature of the spins. Our results enhance our understanding of soft modes in topological frustrated magnets that drive both the unusual physics of quantum dipolar systems and future refrigerant material design.