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  • Letter

Dominant Kitaev interaction and field-induced quantum disordered phase in the cobaltate Na2Co2TeO6

Xu-Guang Zhou1,2,3,*, Han Li4,*, Chaebin Kim5,6,*, Akira Matsuo1, Kavita Mehlawat1, Kazuki Matsui1, Zhuo Yang1, Atsuhiko Miyata1, Gang Su7,8 et al.

Koichi Kindo1, Je-Geun Park5,9, Yoshimitsu Kohama1,†, Wei Li7,‡, and Yasuhiro H. Matsuda1,§

  • *These authors contributed equally to this work.
  • †Contact author: ykohama@g.ecc.u-tokyo.ac.jp
  • ‡Contact author: w.li@itp.ac.cn
  • §Contact author: ymatsuda@issp.u-tokyo.ac.jp

Phys. Rev. B 112, L241108 – Published 5 December, 2025

DOI: https://doi.org/10.1103/r574-yrrp

Abstract

The identification of quantum spin-liquid phases in Kitaev candidate materials remains a major experimental challenge. Since most Kitaev candidates develop antiferromagnetic (AFM) order at low temperatures, currently there is great interest on the field-induced magnetic disordered phase in these compounds that are distinct from (partially) polarized states. Recently, a cobaltate Na2Co2TeO6 has emerged as a promising Kitaev candidate with high-spin t2g5eg2 configuration and spin-orbit-entangled Jeff=1/2 honeycomb lattice system. There are intensive studies on field-induced magnetic states and phase transitions under in-plane magnetic fields. In this study, we propose an intermediate disordered phase induced by an out-of-plane field along the c-axis, through high-field magnetization and magnetocaloric effect measurements. To explain the high-field behavior of Na2Co2TeO6, we develop an effective K−J−Γ−Γ′ spin model featuring a dominant AFM Kitaev interaction. This framework uncovers an intermediate quantum spin-liquid phase, establishing the material as a unique platform for exploring Kitaev physics and field-induced quantum-disordered states.

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