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    Strongly correlated topological surface states in the type-II Dirac semimetal NiTe2

    Neeraj Bhatt, Asif Ali, Deepali Sharma, Sakshi Bansal, Manasi Mandal, Ravi Prakash Singh, and Ravi Shankar Singh*

    • *Contact author: rssingh@iiserb.ac.in

    Phys. Rev. B 111, 245157 – Published 25 June, 2025

    DOI: https://doi.org/10.1103/qklp-cn3m

    Abstract

    Nontrivial topology in type-II Dirac semimetal NiTe2 leading to topologically protected surface states gives rise to fascinating phenomena holding great promise for next-generation electronic and spintronic devices. Key parameters such as lattice parameter, disorder, vacancies, and electron correlation, significantly influence the electronic structure and, subsequently, the physical properties. To resolve the discrepancy between the theoretical description and experimentally observed topological surface states, we comprehensively investigate the electronic structure of NiTe2 using angle-resolved photoemission spectroscopy and density functional theory. Although the bulk electronic structure is found to be well described within mean-field approaches, an accurate description of topological surface states is obtained only by incorporating surface electronic correlation. We reveal that the strongly correlated surface states forming Dirac-like conical crossing much below Fermi level have hybridized Ni3d and Te5p character. These findings underscore the intricate interplay between electron correlation and band topology, broadening our understanding of many-body correlation effects on the topological surface states in quantum materials.

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