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    Observation of Zeeman splitting in the spin-polarized chiral fermion state in the Weyl semimetal TaAs

    H. Murakawa1,*, M. Komada1,†, D.-A. Deaconu2, M. S. Bahramy2, R. V. Belosludov3, T. Kida4, M. Hagiwara4, H. Sakai1, and N. Hanasaki1,5

    • 1Department of Physics, The University of Osaka, Toyonaka, Osaka 560-0043, Japan
    • 2Department of Physics and Astronomy, University of Manchester, Oxford Road, Manchester M13 9PL, United Kingdom
    • 3Institute for Materials Research, Tohoku University, Aoba-ku, Sendai 980-8577, Japan
    • 4Center for Advanced High Magnetic Field Science (AHMF), Graduate School of Science, The University of Osaka, Toyonaka, Osaka 560-0043, Japan
    • 5Spintronics Research Network Division, Institute for Open and Transdisciplinary Research Initiatives, The University of Osaka, Suita, Osaka 565-0871, Japan

    • *Contact author: murakawa@phys.sci.osaka-u.ac.jp
    • †Contact author: komada@gmr.phys.sci.osaka-u.ac.jp

    Phys. Rev. B 112, 045117 – Published 10 July, 2025

    DOI: https://doi.org/10.1103/qjt5-x6p4

    Abstract

    We report a spin-polarized chiral fermion state in the prototypical Weyl semimetal TaAs through a combination of Shubnikov-de Haas (SdH) oscillation measurements and Density functional theory (DFT) calculations. Our first-principles calculations reveal that the Fermi pockets surrounding neighboring Weyl nodes are strongly spin-polarized with opposite chiralities, arising from the interplay between spin-orbit coupling, spatial inversion asymmetry, and the crystalline mirror symmetries of the TaAs lattice. When subjected to an external magnetic field, they are observed to undergo a distinct Zeeman splitting, appearing as pronounced SdH oscillations, whose amplitude and frequencies can significantly vary depending on the direction of the magnetic field in the mirror planes protecting the chiralities of the Weyl nodes.

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