Evolution of the 1/9 magnetization plateau in the kagome system
Phys. Rev. B 114, 134407 – Published 8 September, 2026
DOI: https://doi.org/10.1103/q3yj-t2hj
Abstract
The 1/9 magnetization plateau has recently been observed in the spin-1/2 kagome Heisenberg antiferromagnet (KHA) (YCOB), a promising quantum spin liquid (QSL) candidate. However, the 1/9 plateau has so far been reported only in YCOB, and its microscopic origin and low-energy nature remain under debate. In this study, we investigate the magnetic properties of the chlorine-substituted series (YCOB-Cl) and track the evolution of the 1/9 magnetization plateau across the doping series. We observe clear signatures of the 1/9 plateau at multiple nominal Cl concentrations. The temperature dependence of the plateau response evolves systematically with increasing , consistent with a progressive suppression of low-energy spectral weight and the emergence of a possible effective gap scale. Complementary magnetic torque measurements further show that the magnetic oscillations accompanying the plateau are present only in the sample, indicating that chemical substitution strongly affects the low-energy states associated with the plateau. Taken together, our results establish YCOB-Cl as a tunable platform for exploring how chemical disorder and modified exchange networks reshape the 1/9 plateau and its associated anomalous magnetic responses.