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    Evolution of the 1/9 magnetization plateau in the kagome system YCu3(OH)6[(ClxBr1−x)3−y(OH)y]

    Guoxin Zheng1, Yuan Zhu1, Noah West1, Kaila Jenkins1, Dechen Zhang1, Kuan-Wen Chen1, Aaron Chan1, Zhenyuan Zeng2,3, Aini Xu2,3 et al.

    Oscar A. Valenzuela4, Joanna Blawat4, John Singleton4, Patrick A. Lee5, Shiliang Li2,3,6, and Lu Li1,*

    • *Contact author: luli@umich.edu

    Phys. Rev. B 114, 134407 – Published 8 September, 2026

    DOI: https://doi.org/10.1103/q3yj-t2hj

    Abstract

    The 1/9 magnetization plateau has recently been observed in the spin-1/2 kagome Heisenberg antiferromagnet (KHA) YCu3(OH)6Br2[Br1−y(OH)y] (YCOB), a promising quantum spin liquid (QSL) candidate. However, the 1/9 plateau has so far been reported only in YCOB, and its microscopic origin and low-energy nature remain under debate. In this study, we investigate the magnetic properties of the chlorine-substituted series YCu3(OH)6[(ClxBr1−x)3−y(OH)y] (YCOB-Cl) and track the evolution of the 1/9 magnetization plateau across the doping series. We observe clear signatures of the 1/9 plateau at multiple nominal Cl concentrations. The temperature dependence of the plateau response evolves systematically with increasing x, consistent with a progressive suppression of low-energy spectral weight and the emergence of a possible effective gap scale. Complementary magnetic torque measurements further show that the magnetic oscillations accompanying the plateau are present only in the x=0 sample, indicating that chemical substitution strongly affects the low-energy states associated with the plateau. Taken together, our results establish YCOB-Cl as a tunable platform for exploring how chemical disorder and modified exchange networks reshape the 1/9 plateau and its associated anomalous magnetic responses.

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