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Plasmonic detection of Rashba spin-orbit coupling in monolayer transition metal dichalcogenides

Y. Li1,2, Z. H. Tao2,*, Y. M. Xiao1,†, W. Xu1,3,‡, Q. N. Li1, F. M. Peeters2,4, D. Neilson2, and M. V. Milošević2,§

  • 1School of Physics and Astronomy, Yunnan University, Kunming 650091, People's Republic of China
  • 2Department of Physics and NANOlight Center of Excellence, University of Antwerp, Groenenborgerlaan 171, 2020 Antwerp, Belgium
  • 3Key Laboratory of Materials Physics, Institute of Solid State Physics, HFIPS, Chinese Academy of Sciences, Hefei 230031, People's Republic of China
  • 4Departamento de Física, Universidade Federal do Ceará, Caixa Postal 6030, Campus do Pici, 60455-900 Fortaleza, Ceará, Brazil

  • *Contact author: zehua.tao@uantwerpen.be
  • †Contact author: yiming.xiao@ynu.edu.cn
  • ‡Contact author: wenxu_issp@aliyun.com
  • §Contact author: milorad.milosevic@uantwerpen.be

Phys. Rev. B 112, L161404 – Published 10 October, 2025

DOI: https://doi.org/10.1103/pxkx-rvkl

Abstract

Rashba spin-orbit coupling (RSOC) induces strong momentum-dependent spin splitting and plays a crucial role in fields such as spintronics and topological photonics. We here theoretically investigate the collective excitations in monolayer transition-metal dichalcogenides (ML-TMDs) hosting RSOC, and conceive an approach to precisely quantify the strength of RSOC using plasmons. We determine the electron energy loss function (EELF) and plasmon dispersions for n-type ML-TMDs from the dynamic dielectric function in the framework of the standard random phase approximation. In this system, both optical and acoustic plasmon modes are observed in the EELF and plasmon dispersions. Moreover, the plasmonic and spectral properties are tunable by electron density and dependent on RSOC. Crucially, we identify a minimum energy gap between the two plasmon modes to serve as a direct spectral signature of the RSOC strength. These results establish plasmons as a noninvasive, precise, and broadly tunable technique for determining RSOC in TMD van der Waals heterostructures and devices.

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