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  • Letter

Unidirectional charge and pair density waves in topological monolayer 1T′−MoTe2

Li-Xuan Wei1,*, Peng-Cheng Xiao2,*, Fangsen Li3,*, Li Wang3, Bo-Yuan Deng3, Fang-Jun Cheng1, Fa-Wei Zheng4, Ning Hao5, Ping Zhang2,6,† et al.

Xu-Cun Ma1,7,‡, Qi-Kun Xue1,7,8,9,10, and Can-Li Song1,7,§

  • *These authors contributed equally to this work.
  • †Contact author: zhang_ping@iapcm.ac.cn
  • ‡Contact author: xucunma@mail.tsinghua.edu.cn
  • §Contact author: clsong07@mail.tsinghua.edu.cn

Phys. Rev. B 112, L060503 – Published 13 August, 2025

DOI: https://doi.org/10.1103/px77-3gg1

Abstract

Symmetry-breaking phenomena are identifiable in numerous strongly correlated systems including high-temperature superconductors. However, identification of these exotic states and understanding their interplay with superconductivity in topological materials remains limited. Here we employ cryogenic scanning tunneling microscopy to reveal coexistent charge and pair density waves (CDWs and PDWs) in topological monolayer 1T′−MoTe2. The two orders are modulated unidirectionally and share the same periodicity of five unit cells or a wave vector near (0, 0.4)π/b (b is the lattice constant along the zigzag Mo chains). Importantly, the PDW features a two-gap superconductivity below a transition temperature of around 6.0 K and induces a unique secondary particle-hole-symmetric CDW at twice its wave vector. Combining these results and our density functional calculations, we elucidate that the two unidirectional orders are driven by nesting behaviors between electron and hole pockets. Our findings establish monolayer 1T′−MoTe2 as a topological paradigm to explore multiple preexisting symmetry-breaking states.

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