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    Magnetic states of Fe and Co atoms in helimagnetic Fe1−xCoxGe (0≤ x ≤0.3) studied by Fe57, Co59 NMR spectroscopy

    Z. N. Volkova1,2, V. V. Ogloblichev1, A. V. Bokov2, and A. V. Tsvyashchenko2

    Phys. Rev. B 114, 214423 – Published 20 October, 2026

    DOI: https://doi.org/10.1103/pwrm-5hw8

    Abstract

    The results of a study of Fe1−xCoxGe(0≤x≤0.3) compounds using nuclear magnetic resonance (NMR) spectroscopy on the nuclei of Fe57 and Co59 in helical spin ordered state are represented in this paper. It was established that cobalt atoms are randomly distributed within the crystal structure of Fe1−xCoxGe. The hyperfine fields and magnetic moments for iron and cobalt atoms were determined at a temperature of T=4.2K. The average Fe magnetic moment decreases from 0.9 μB (for x=0) to 0.85 μB (for x=0.3), whereas the Co magnetic moment is of about zero. It is shown that the hyperfine fields induced at the Co nuclei by Fe atoms arise from the strong hybridization of the Fe 3d and Co 3d orbitals.

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