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    Spin-dependent orbital selectivity and partial Kondo-like screening in the magnetically ordered Hund's metal Sr2CoO4

    Shivani Bhardwaj*

    Sudhir K. Pandey†

    • *Contact author: sbhardwajiitm369@gmail.com
    • †Contact author: sudhir@iitmandi.ac.in

    Phys. Rev. B 113, 235147 – Published 24 June, 2026

    DOI: https://doi.org/10.1103/nyr5-84k4

    Abstract

    Hund's metallicity in 3d transition metal oxides constitutes a rare class of compounds, since they have been long understood considering the dominance of Hubbard U. LiV2O4and Sr2CoO4 belong to this rare class of metals; among them, LiV2O4 has been the subject of extensive investigations for its unconventional heavy-fermion behavior, while studies on Sr2CoO4 remain limited despite its anomalous ferromagnetic ground state. In this study, we report an unusual spin-orbital selective localization in Sr2CoO4 consistent with a Kondo-like resonance at ∼70K in the spin-up channel of orbitals of t2g symmetry using a combination of Density functional theory and Dynamical mean-field theory calculations. Correspondingly, an appreciable reduction in the magnetization below T=100K is further suggestive of a partial Kondo-like screening of local moments active at low temperatures, providing a plausible explanation for its effective spin magnetization state and upturn in its resistivity observed in experimental reports. We note a significant effect of Hund's induced spin-orbital selective incoherence in dictating the temperature evolution of its macroscopic observables e.g., spin-spin correlation function and effective local moment. Our results reveal a potentially distinct/new form of spin-dependent selectivity induced via Hund's coupling in addition to the conventional orbital-selectivity in the Hund's metals, as a plausible key mechanism in stabilizing their long-range magnetic order.

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