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    Polarization engineering of the orbital Hall conductivity in the two-dimensional ferroelectric higher-order topological insulators Tl2S and SnS

    Yingjie Hu1, Heng Gao1,*, Yabei Wu2,†, and Wei Ren1,‡

    • 1Physics Department, Materials Genome Institute, Institute for Quantum Science and Technology, Shanghai Key Laboratory of High Temperature Superconductors, Shanghai University, Shanghai 200444, China
    • 2Department of Materials Science and Engineering and Guangdong Provincial Key Lab for Computational Science and Materials Design, Southern University of Science and Technology, Shenzhen, Guangdong 518055, China

    • *Contact author: gaoheng@shu.edu.cn
    • †Contact author: wuyb3@sustech.edu.cn
    • ‡Contact author: renwei@shu.edu.cn

    Phys. Rev. B 114, 125132 – Published 26 August, 2026

    DOI: https://doi.org/10.1103/nqkg-2sj7

    Abstract

    Ferroelectric higher-order topological insulators (HOTIs) exhibit versatile physical properties arising from the interplay between ferroelectric polarization and band topology. This work investigates the topological origin of two classes of two-dimensional (2D) ferroelectric HOTIs with out-of-plane or in-plane polarization, revealing their orbital transport behaviors and the distinct mechanism for engineering orbital Hall conductivity (OHC) via polarization control. Our results demonstrate the unique role of polarization in modulating both the higher-order band topology and orbital transport. A strong coupling between in-plane polarization and higher-order topology is identified, establishing in-plane polarization as an intrinsic means to modulate the OHC plateau within the band gap. Using Tl2S and SnS as representative models of the two HOTI types, we demonstrate persistent and electrically tunable orbital transport, respectively. Our study advances the understanding of the coupling among ferroelectricity, higher-order topology, and orbital transport, offering alternative avenues for controllable orbitronics.

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