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    Inelastic neutron scattering signatures of chiral phonons

    Tingting Wang1, Jun Zhou1, Qingyong Ren2,3,4,*, and Lifa Zhang1,†

    • 1Ministry of Education Key Laboratory of NSLSCS, Phonon Engineering Research Center of Jiangsu Province, Center for Quantum Transport and Thermal Energy Science, Institute of Physics Frontiers and Interdisciplinary Sciences, School of Physics and Technology, Nanjing Normal University, Nanjing 210023, China
    • 2Institute of High Energy Physics, Chinese Academy of Sciences, Beijing 100049, China
    • 3Spallation Neutron Source Science Center, Dongguan 523803, China
    • 4Guangdong Provincial Key Laboratory of Extreme Conditions, Dongguan 523803, China

    • *Contact author: renqy@ihep.ac.cn
    • †Contact author: phyzlf@njnu.edu.cn

    Phys. Rev. B 114, 034302 – Published 6 July, 2026

    DOI: https://doi.org/10.1103/nmdy-9tkl

    Abstract

    Chiral phonons endow lattice vibrations with angular momentum and can give rise to phonon magnetism, offering routes to control magnetism and topology. However, experimentally resolving their polarization, handedness, and magnetism across the Brillouin zone remains challenging. Here, we formulate a measurement-oriented inelastic neutron scattering (INS) framework to diagnose these attributes from the nuclear one-phonon response in the scattering readout. We demonstrate that angular intensity fingerprints classify linear, elliptical, and circular polarizations, while phase-sensitive time-resolved signatures provide a benchmark readout of handedness. Furthermore, we show that phonon magnetic moments manifest as characteristic spectral splittings and intensity redistributions under external fields. Benchmarked in chiral Te and paramagnetic CeF3, this framework provides a comprehensive momentum-resolved probe for the geometric and magnetic nature of chiral phonons.

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