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Attaining the ground state of kagome artificial spin ice via ultrafast site-specific laser annealing

D. Pecchio, S. Sahoo*, V. Scagnoli†, and L. J. Heyderman‡

  • *Contact author: sourav.sahoo@psi.ch
  • †Contact author: valerio.scagnoli@psi.ch
  • ‡Contact author: laura.heyderman@psi.ch

Phys. Rev. B 113, 054434 – Published 20 February, 2026

DOI: https://doi.org/10.1103/nl4z-3pn1

Abstract

Artificial spin ices (ASIs) provide a versatile platform to explore magnetic frustration and emergent phenomena. However, in kagome ASI, experimental access to the ground state remains elusive due to dynamical freezing. Here we demonstrate a deterministic and rewritable approach to attain the ground state using ultrafast, site-selective laser annealing. By engineering sublattice-dependent optical absorption through selective capping of the nanomagnets with Cr or utilizing different nanomagnet thicknesses, we achieve selective partial demagnetization and subsequent reversal of one nanomagnet sublattice under a subcoercive magnetic field, driving the system into the ground state in a single switching step. Magnetic force microscopy reveals nearly perfect long-range ordering, while heat-transfer simulations confirm the sublattice-selective excitation mechanism. This work establishes an ultrafast method to attain the kagome ASI ground state, which does not require a modification of the geometry of the ASI or the materials used for the individual nanomagnets. Beyond ground-state writing, this site-selective activation provides an important tool for controlling the magnetic states, which is important for applications such as reconfigurable magnonic crystals, neuromorphic computing and programmable nanomagnetic logic.

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References (48)

  1. S. H. Skjærvø, C. H. Marrows, R. L. Stamps, and L. J. Heyderman, Advances in artificial spin ice, Nat. Rev. Phys. 2, 13 (2020).
  2. M. J. Harris, S. T. Bramwell, D. F. McMorrow, T. Zeiske, and K. W. Godfrey, Geometrical frustration in the ferromagnetic pyrochlore Ho2Ti2O7, Phys. Rev. Lett. 79, 2554 (1997).
  3. S. Ladak, D. E. Read, G. K. Perkins, L. F. Cohen, and W. R. Branford, Direct observation of magnetic monopole defects in an artificial spin-ice system, Nat. Phys. 6, 359 (2010).
  4. E. Mengotti, L. J. Heyderman, A. F. Rodríguez, F. Nolting, R. V. Hügli, and H.-B. Braun, Real-space observation of emergent magnetic monopoles and associated Dirac strings in artificial kagome spin ice, Nat. Phys. 7, 68 (2011).
  5. L. Anghinolfi, H. Luetkens, J. Perron, M. G. Flokstra, O. Sendetskyi, A. Suter, T. Prokscha, P. M. Derlet, S. L. Lee, and L. J. Heyderman, Thermodynamic phase transitions in a frustrated magnetic metamaterial, Nat. Commun. 6, 8278 (2015).
  6. O. Sendetskyi, L. Anghinolfi, V. Scagnoli, G. Möller, N. Leo, A. Alberca, J. Kohlbrecher, J. Lüning, U. Staub, and L. J. Heyderman, Magnetic diffuse scattering in artificial kagome spin ice, Phys. Rev. B 93, 224413 (2016).
  7. O. Sendetskyi, V. Scagnoli, N. Leo, L. Anghinolfi, A. Alberca, J. Lüning, U. Staub, P. M. Derlet, and L. J. Heyderman, Continuous magnetic phase transition in artificial square ice, Phys. Rev. B 99, 214430 (2019).
  8. M. Goryca, X. Zhang, J. D. Watts, C. Nisoli, C. Leighton, P. Schiffer, and S. A. Crooker, Magnetic field–dependent thermodynamic properties of square and quadrupolar artificial spin ice, Phys. Rev. B 105, 094406 (2022).
  9. R. F. Wang, C. Nisoli, R. S. Freitas, J. Li, W. McConville, B. J. Cooley, M. S. Lund, N. Samarth, C. Leighton, V. H. Crespi, and P. Schiffer, Artificial ‘spin ice’ in a geometrically frustrated lattice of nanoscale ferromagnetic islands, Nature (Lond.) 439, 303 (2006).
  10. C. Nisoli, Frustration(s) and the ice rule: From natural materials to the deliberate design of exotic behaviors, in Frustrated Materials and Ferroic Glasses, edited by T. Lookman, and X. Ren, Vol. 275 (Springer International Publishing, Cham, 2018), pp. 57–99.
  11. E. Mengotti, L. J. Heyderman, A. Fraile Rodríguez, A. Bisig, L. Le Guyader, F. Nolting, and H. B. Braun, Building blocks of an artificial kagome spin ice: Photoemission electron microscopy of arrays of ferromagnetic islands, Phys. Rev. B 78, 144402 (2008).
  12. M. Tanaka, E. Saitoh, H. Miyajima, T. Yamaoka, and Y. Iye, Magnetic interactions in a ferromagnetic honeycomb nanoscale network, Phys. Rev. B 73, 052411 (2006).
  13. Y. Qi, T. Brintlinger, and J. Cumings, Direct observation of the ice rule in an artificial kagome spin ice, Phys. Rev. B 77, 094418 (2008).
  14. G. Möller and R. Moessner, Magnetic multipole analysis of kagome and artificial spin-ice dipolar arrays, Phys. Rev. B 80, 140409(R) (2009).
  15. G.-W. Chern, P. Mellado, and O. Tchernyshyov, Two-stage ordering of spins in dipolar spin ice on the kagome lattice, Phys. Rev. Lett. 106, 207202 (2011).
  16. G.-W. Chern and O. Tchernyshyov, Magnetic charge and ordering in kagome spin ice, Philos. Trans. R. Soc. Math. Phys. Eng. Sci. 370, 5718 (2012).
  17. C. Castelnovo, R. Moessner, and S. L. Sondhi, Magnetic monopoles in spin ice, Nature (Lond.) 451, 42 (2008).
  18. A. Farhan, P. M. Derlet, L. Anghinolfi, A. Kleibert, and L. J. Heyderman, Magnetic charge and moment dynamics in artificial kagome spin ice, Phys. Rev. B 96, 064409 (2017).
  19. N. Rougemaille, F. Montaigne, B. Canals, A. Duluard, D. Lacour, M. Hehn, R. Belkhou, O. Fruchart, S. El Moussaoui, A. Bendounan, and F. Maccherozzi, Artificial kagome arrays of nanomagnets: A frozen dipolar spin ice, Phys. Rev. Lett. 106, 057209 (2011).
  20. F. Montaigne, D. Lacour, I. A. Chioar, N. Rougemaille, D. Louis, S. M. Murtry, H. Riahi, B. S. Burgos, T. O. Menteş, A. Locatelli, B. Canals, and M. Hehn, Size distribution of magnetic charge domains in thermally activated but out-of-equilibrium artificial spin ice, Sci. Rep. 4, 5702 (2014).
  21. S. Zhang, I. Gilbert, C. Nisoli, G.-W. Chern, M. J. Erickson, L. O’Brien, C. Leighton, P. E. Lammert, V. H. Crespi, and P. Schiffer, Crystallites of magnetic charges in artificial spin ice, Nature (Lond.) 500, 553 (2013).
  22. V. Schánilec, B. Canals, V. Uhlíř, L. Flajšman, J. Sadílek, T. Šikola, and N. Rougemaille, Bypassing dynamical freezing in artificial kagome ice, Phys. Rev. Lett. 125, 057203 (2020).
  23. J. Drisko, T. Marsh, and J. Cumings, Topological frustration of artificial spin ice, Nat. Commun. 8, 14009 (2017).
  24. J. Drisko, FePd3 as a material for studying thermally active artificial spin ice systems, Phys. Rev. B 91, 224406 (2015).
  25. K. Hofhuis, A. Hrabec, H. Arava, N. Leo, Y.-L. Huang, R. V. Chopdekar, S. Parchenko, A. Kleibert, S. Koraltan, C. Abert, C. Vogler, D. Suess, P. M. Derlet, and L. J. Heyderman, Thermally superactive artificial kagome spin ice structures obtained with the interfacial Dzyaloshinskii-Moriya interaction, Phys. Rev. B 102, 180405 (2020).
  26. K. Hofhuis, S. H. Skjærvø, S. Parchenko, H. Arava, Z. Luo, A. Kleibert, P. M. Derlet, and L. J. Heyderman, Real-space imaging of phase transitions in bridged artificial kagome spin ice, Nat. Phys. 18, 699 (2022).
  27. W.-C. Yue, Z. Yuan, Y.-Y. Lyu, S. Dong, J. Zhou, Z.-L. Xiao, L. He, X. Tu, Y. Dong, H. Wang, W. Xu, L. Kang, P. Wu, C. Nisoli, W.-K. Kwok, and Y.-L. Wang, Crystallizing kagome artificial spin ice, Phys. Rev. Lett. 129, 057202 (2022).
  28. J. Gartside, D. Arroo, D. Burn, V. Bemmer, A. Moskalenko, L. Cohen, and W. Branford, Realization of ground state in artificial kagome spin ice via topological defect-driven magnetic writing, Nat. Nanotechnol. 13, 53 (2018).
  29. V. M. Parakkat, G. M. Macauley, R. L. Stamps, and K. M. Krishnan, Configurable artificial spin ice with site-specific local magnetic fields, Phys. Rev. Lett. 126, 017203 (2021).
  30. R. V. Hügli, G. Duff, B. O’Conchuir, E. Mengotti, A. F. Rodríguez, F. Nolting, L. J. Heyderman, and H. B. Braun, Artificial kagome spin ice: Dimensional reduction, avalanche control and emergent magnetic monopoles, Philos. Trans. R. Soc. Math. Phys. Eng. Sci. 370, 5767 (2012).
  31. R. V. Chopdekar, G. Duff, R. V. Hügli, E. Mengotti, D. A. Zanin, L. J. Heyderman, and H. B. Braun, Controlling vortex chirality in hexagonal building blocks of artificial spin ice, New J. Phys. 15, 125033 (2013).
  32. S. N. Panda, S. Mondal, S. Majumder, and A. Barman, Ultrafast demagnetization and precession in permalloy films with varying thickness, Phys. Rev. B 108, 144421 (2023).
  33. Z. Liang, T. Bu, Z. Lyu, Z. Liu, A. Hrabec, L. Wang, Y. Dou, J. Ding, P. Ge, W. Yang, T. Huang, J. Yang, L. J. Heyderman, Y. Liu, Z. Yu, and Z. Luo, Ultrafast probabilistic neuron in an artificial spin ice for robust deep neural networks, Adv. Funct. Mater. 35, 2417334 (2025).
  34. D. Pecchio, S. Sahoo, O. Chubykalo-Fesenko, S. Koraltan, G. M. Macauley, T. Thomson, D. Suess, V. Scagnoli, and L. J. Heyderman, Ultrafast laser-induced magnetic relaxation in artificial spin ice driven by dipolar interactions, Phys. Rev. B 113, 064404 (2026).
  35. S. A. Daunheimer, Reducing disorder in artificial kagome ice, Phys. Rev. Lett. 107, 167201 (2011).
  36. Z. Budrikis, J. P. Morgan, J. Akerman, A. Stein, P. Politi, S. Langridge, C. H. Marrows, and R. L. Stamps, Disorder strength and field-driven ground state domain formation in artificial spin ice: Experiment, simulation, and theory, Phys. Rev. Lett. 109, 037203 (2012).
  37. Z. Budrikis, P. Politi, and R. L. Stamps, A network model for field and quenched disorder effects in artificial spin ice, New J. Phys. 14, 045008 (2012).
  38. J. M. Porro, A. Bedoya-Pinto, A. Berger, and P. Vavassori, Exploring thermally induced states in square artificial spin-ice arrays, New J. Phys. 15, 055012 (2013).
  39. A. Farhan, P. M. Derlet, A. Kleibert, A. Balan, R. V. Chopdekar, M. Wyss, J. Perron, A. Scholl, F. Nolting, and L. J. Heyderman, Direct observation of thermal relaxation in artificial spin ice, Phys. Rev. Lett. 111, 057204 (2013).
  40. X. Zhang, Y. Lao, J. Sklenar, N. S. Bingham, J. T. Batley, J. D. Watts, C. Nisoli, C. Leighton, and P. Schiffer, Understanding thermal annealing of artificial spin ice, APL Mater. 7, 111112 (2019).
  41. B. Canals, I.-A. Chioar, V.-D. Nguyen, M. Hehn, D. Lacour, F. Montaigne, A. Locatelli, T. O. Menteş, B. S. Burgos, and N. Rougemaille, Fragmentation of magnetism in artificial kagome dipolar spin ice, Nat. Commun. 7, 11446 (2016).
  42. R. F. Wang, J. Li, W. McConville, C. Nisoli, X. Ke, J. W. Freeland, V. Rose, M. Grimsditch, P. Lammert, V. H. Crespi, and P. Schiffer, Demagnetization protocols for frustrated interacting nanomagnet arrays, J. Appl. Phys. 101, 09J104 (2007).
  43. J. P. Morgan, A. Bellew, A. Stein, S. Langridge, and C. Marrows, Linear field demagnetization of artificial magnetic square ice, Front. Phys. 1, 28 (2013).
  44. X. Ke, Energy minimization and AC demagnetization in a nanomagnet array, Phys. Rev. Lett. 101, 037205 (2008).
  45. F. Garcia, J. Sort, B. Rodmacq, S. Auffret, and B. Dieny, Large anomalous enhancement of perpendicular exchange bias by introduction of a nonmagnetic spacer between the ferromagnetic and antiferromagnetic layers, Appl. Phys. Lett. 83, 3537 (2003).
  46. I. Theodorakos, I. Zergioti, V. Vamvakas, D. Tsoukalas, and Y. S. Raptis, Picosecond and nanosecond laser annealing and simulation of amorphous silicon thin films for solar cell applications, J. Appl. Phys. 115, 043108 (2014).
  47. B. J. Simonds, S. Misra, N. Paudel, K. Vandewal, A. Salleo, C. Ferekides, and M. A. Scarpulla, Near infrared laser annealing of CdTe and in-situ measurement of the evolution of structural and optical properties, J. Appl. Phys. 119, 165305 (2016).
  48. V. Scagnoli, Data supporting “Attaining the ground state of Kagome artificial spin ice via ultrafast site-specific laser annealing,” [Data set], Zenodo (2025), doi:10.5281/zenodo.17967151.

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