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    Quantum melting of spin-1 dimer solid induced by interchain couplings

    Yi Xu (徐熠)1,*, Tianfu Fu1, Juraj Hasik2,3,4,†, and Andriy H. Nevidomskyy1,5,6,‡

    • *Contact author: slowlight@rice.edu
    • †Contact author: j.hasik@uva.nl
    • ‡Contact author: nevidomskyy@rice.edu

    Phys. Rev. B 114, 034418 – Published 17 July, 2026

    DOI: https://doi.org/10.1103/nd9v-xf1d

    Abstract

    Dimerized valence bond solids appear naturally in spin-1/2 systems on bipartite lattices, with the geometric frustrations playing a key role both in their stability and the eventual melting due to quantum fluctuations. Here, we ask the question of the stability of such dimerized solids in spin-1 systems, taking the anisotropic square lattice with bilinear and biquadratic spin-spin interactions as a paradigmatic model. The lattice can be viewed as a set of coupled spin-1 chains, which in the limit of vanishing interchain coupling are known to possess a stable dimer phase. We study this model using the density matrix renormalization group (DMRG) and infinite projected entangled-pair states (iPEPS) techniques, supplemented by the analytical mean-field and linear flavor-wave theory calculations. While the latter predicts the dimer phase to remain stable up to a reasonably large interchain-to-intrachain coupling ratio r≲0.6, the DMRG and iPEPS find that the dimer solid melts for much weaker interchain coupling not exceeding r≲0.15. We find the transition into a magnetically ordered state to be first order, manifested by a hysteresis and order parameter jump, precluding the deconfined quantum critical scenario. The apparent lack of stability of dimerized phases in 2D spin-1 systems is indicative of strong quantum fluctuations that melt the dimer solid.

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