Tracking doublon-holon dynamics in high-harmonic generation from Mott insulators
Phys. Rev. B 113, 245147 – Published 26 June, 2026
DOI: https://doi.org/10.1103/n4gk-jxpc
Abstract
High-harmonic generation (HHG) in strongly correlated Mott insulators is investigated using exact diagonalization and time-dependent density-matrix propagation of a laser-driven one-dimensional Hubbard chain. By projecting onto equilibrium Hubbard bands, we use the doublon population and its dynamics as a diagnostic to analyze intraband (spin-wave-like) and interband (doublon-holon creation) excitation channels. A filling-dependent crossover emerges: Bloch-like intraband response at dilute filling, mixed dynamics at intermediate filling, and interband-dominated HHG with plateau and cutoff near half-filling. In the considered parameter range, increasing interaction strength strongly suppresses interband contributions through the enlarged Mott gap and correlation-induced localization. Intra- and interband current decomposition reveals opposing flows below the Mott gap () and selective dephasing suppression of interband coherence, enhancing net doublon accumulation. Time-frequency analysis uncovers the filling-dependent features of quantum trajectories, manifesting in distinct below- emission. This doublon-based analysis provides a transparent link between equilibrium spin-charge separation and nonequilibrium strong-field response, and clarifies how dephasing modifies interband coherence and doublon accumulation.