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    Tracking doublon-holon dynamics in high-harmonic generation from Mott insulators

    Tao-Yuan Du1,*, Hui-Ru Li1, Bo Li1, and Ruifeng Lu2,†

    • *Contact author: duty710@163.com
    • †Contact author: rflu@njust.edu.cn

    Phys. Rev. B 113, 245147 – Published 26 June, 2026

    DOI: https://doi.org/10.1103/n4gk-jxpc

    Abstract

    High-harmonic generation (HHG) in strongly correlated Mott insulators is investigated using exact diagonalization and time-dependent density-matrix propagation of a laser-driven one-dimensional Hubbard chain. By projecting onto equilibrium Hubbard bands, we use the doublon population and its dynamics as a diagnostic to analyze intraband (spin-wave-like) and interband (doublon-holon creation) excitation channels. A filling-dependent crossover emerges: Bloch-like intraband response at dilute filling, mixed dynamics at intermediate filling, and interband-dominated HHG with plateau and cutoff near half-filling. In the considered parameter range, increasing interaction strength U strongly suppresses interband contributions through the enlarged Mott gap and correlation-induced localization. Intra- and interband current decomposition reveals opposing flows below the Mott gap (ΔMott) and selective dephasing suppression of interband coherence, enhancing net doublon accumulation. Time-frequency analysis uncovers the filling-dependent features of quantum trajectories, manifesting in distinct below-ΔMott emission. This doublon-based analysis provides a transparent link between equilibrium spin-charge separation and nonequilibrium strong-field response, and clarifies how dephasing modifies interband coherence and doublon accumulation.

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