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    Electronic transport, thermal transport, thermal expansion, and magnetization in the strongly correlated metal LaNiO3

    J.-S. Zhou1,*, B. Dabrowski2, J. F. Mitchell3, and M. D. Johannes4

    • *Contact author: jszhou@mail.utexas.edu

    Phys. Rev. B 113, 035115 – Published 7 January, 2026

    DOI: https://doi.org/10.1103/n2jd-q5q2

    Abstract

    Perovskite structured LaNiO3 is a strongly correlated metal with intriguing thermal and magnetic properties. The volume dependence of calculated and measured physical properties can add additional critical information to develop a more in-depth understanding of this strongly correlated phenomenon. Taking advantage of recent single crystal LaNiO3 growth using the floating-zone method, we have measured the thermal expansion, the magnetostriction, and the pressure dependence of the magnetic susceptibility, which then allows derivation of the Grüneisen parameters γe=dlnN(EF)dlnV, γχ=dlnχdlnV, as well as of electric and thermal transport properties. We simulate the volume dependence of structural and magnetic properties using Density Functional Theory calculations at the Generalized Gradient Approximation level. A large discrepancy between experimental values and calculated ones suggests that strong correlations are likely to be dynamic in nature. This study also provides a side-by-side comparison of measurements in single crystal and polycrystalline samples of LaNiO3 to elucidate intrinsic materials properties. A broad hump at high temperatures in the temperature dependence of magnetization found in the single crystal sample of LaNiO3 has been rationalized by a model that includes the influence of electron correlations on the Landau diamagnetism.

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