Motivated by the highest superconducting transition temperature ($T_c$) in multilayer cuprates, we investigated the trilayer Hubbard model by adopting large-scale dynamical cluster quantum Monte Carlo simulations. Focusing on the systems with hole dopings within the two outer layers (OLs) higher than the inner layer (IL), which is believed to be relevant to the realistic multilayer cuprates, our exploration discovered that the IL and OL manifest strong differentiation in a wide range of hole doping combinations. Specifically, the OLs remain metallic while the IL shows a distinct transition from the pseudogap to superconducting state. More importantly, the highest $T_c$ of the composite trilayer system can be largely enhanced compared to the single layer model and the imbalanced hole dopings between IL and OL are generically beneficial for global superconductivity (SC). We further provide strong numerical evidence on the possibility of $d$-wave SC solely hosted in the IL. Our investigation provides insight into the origin of highest $T_c$ in multilayer cuprates.

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• Superconductivity
• Cuprates
• High-temperature superconductors
• Hubbard model
• Monte Carlo methods