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    Photoinduced melting dynamics and collective mode in a correlated charge-ordered system

    Yasuhiro Tanaka1,* and Hitoshi Seo2

    • *Contact author: tanaka.y@neptune.kanazawa-it.ac.jp

    Phys. Rev. B 113, 125129 – Published 16 March, 2026

    DOI: https://doi.org/10.1103/mz8w-3vgz

    Abstract

    We theoretically investigate the transient spectral function during the photoinduced melting of charge order in a correlated electron system, to unravel the dynamical processes triggered by different initial excitations. We employ a one-dimensional interacting spinless fermion model introducing a pulsed laser light, and perform a comparative study by the Hartree-Fock approximation and by the exact diagonalization method to numerically solve the time-dependent Schrödinger equation. We find characteristic behavior in the transient spectral function, whose features strongly depend on the pump light frequency ωp. When ωp is resonant with the collective phase mode of frequency Ωc≃ΔCO/2, where ΔCO is the charge gap, the transient spectral function exhibits a photoinduced in-gap weight that triggers large responses. With increasing laser intensity, the development of in-gap weight directly turns into the collapse of the gap. This charge-order destabilization process is in sharp contrast to the case of ωp>ΔCO, where the photoirradiation induces interband electron-hole excitations giving rise to a shrinkage of the gap. The impact of quantum fluctuations and spatial inhomogeneity on the photoinduced dynamics is also discussed.

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