Photoinduced melting dynamics and collective mode in a correlated charge-ordered system
Phys. Rev. B 113, 125129 – Published 16 March, 2026
DOI: https://doi.org/10.1103/mz8w-3vgz
Abstract
We theoretically investigate the transient spectral function during the photoinduced melting of charge order in a correlated electron system, to unravel the dynamical processes triggered by different initial excitations. We employ a one-dimensional interacting spinless fermion model introducing a pulsed laser light, and perform a comparative study by the Hartree-Fock approximation and by the exact diagonalization method to numerically solve the time-dependent Schrödinger equation. We find characteristic behavior in the transient spectral function, whose features strongly depend on the pump light frequency . When is resonant with the collective phase mode of frequency , where is the charge gap, the transient spectral function exhibits a photoinduced in-gap weight that triggers large responses. With increasing laser intensity, the development of in-gap weight directly turns into the collapse of the gap. This charge-order destabilization process is in sharp contrast to the case of , where the photoirradiation induces interband electron-hole excitations giving rise to a shrinkage of the gap. The impact of quantum fluctuations and spatial inhomogeneity on the photoinduced dynamics is also discussed.