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    Highly fluctuating double-q magnetic order in the van der Waals metal CeTe3

    Ryutaro Okuma1,*, Yuita Fujisawa2, Natsumi Maekawa3, Akiko Nakao4, Yoshihisa Ishikawa4, Riki Kobayashi5, Yoshinori Okada6, and Daichi Ueta7

    • *Contact author: rokuma@issp.u-tokyo.ac.jp

    Phys. Rev. B 114, 024420 – Published 23 July, 2026

    DOI: https://doi.org/10.1103/m9lb-4vhx

    Abstract

    CeTe3 is a van der Waals antiferromagnet composed of magnetic [CeTe]+ layers coupled to highly conducting Te0.5− square nets. Its simple quasi-two-dimensional electronic structure and cleavable nature make it an appealing platform for exploring correlated magnetism in reduced dimensions. To clarify the nature of its low-temperature state, we performed single-crystal neutron diffraction down to 0.3 K, complemented by scanning tunneling microscopy. A magnetic transition near 1.5 K gives rise to incommensurate Bragg peaks at q±∼(±0.17,0,0.31), consistent with a double-q magnetic order whose moments are predominantly aligned along the c axis. The strongly reduced ordered moment is consistent with enhanced quantum fluctuations driven by c−f hybridization, while the deviation of the propagation vectors from simple nesting suggests a coupling to residual charge-density-wave instabilities of the quasi-one-dimensional Te-derived bands. These results indicate that CeTe3 hosts a correlated magnetic ground state where spin and itinerant charge degrees of freedom are intimately linked in the van der Waals limit.

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