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Ferroelastically tunable altermagnets

Ning Ding, Haoshen Ye, Shan-Shan Wang*, and Shuai Dong†

  • Key Laboratory of Quantum Materials and Devices of Ministry of Education, School of Physics, Southeast University, Nanjing 21189, China

  • *Contact author: wangss@seu.edu.cn
  • †Contact author: sdong@seu.edu.cn

Phys. Rev. B 112, L220410 – Published 23 December, 2025

DOI: https://doi.org/10.1103/m33v-xwn3

Abstract

Altermagnets have garnered great interest due to their nonrelativistic spin splitting and unique physical properties. However, the control of altermagnetic states remains underexplored. Here, we propose a multiferroic state, i.e., ferroelastic altermagnetic state, in which ferroelastic strain couples directly to the spin splitting. Through symmetry analysis and first-principles calculations, we identify the ferroelastic d-wave altermagnetism of puckered pentagonal CoSe2 monolayer. Interestingly, uniaxial stress can induce a ferroelastic phase transition, accompanied by a 90∘ rotation of the spin-splitting bands. Cooperative rotation of the lattice and Néel vectors preserves the sign of Kerr angle, whereas noncooperative rotation reverses it. Our work provides a general strategy for manipulating altermagnetism in multiferroic systems and opens other avenues for exploring emergent magnetoelastic phenomena.

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