Leading order coefficients in nonlinear thermoelectric responses with time-reversal symmetry
Phys. Rev. B 114, 115108 – Published 13 August, 2026
DOI: https://doi.org/10.1103/ltrw-mntl
Abstract
In recent years, nonlinear transport phenomena have garnered significant interest in both theoretical explorations and experiments. In this work, we utilize the semiclassical wave-packet theory to calculate disorder-induced second-order transport coefficients: second-order electrical (), thermoelectric (), and thermal () coefficients, capturing the interplay between side-jump and skew-scattering contributions in systems with time-reversal symmetry. By employing a realistic model of topological insulators specifically tailored to represent materials, we quantitatively characterize the Fermi-level dependence of these second-order transport coefficients by explicitly including Coulomb impurity potentials. Furthermore, we elucidate the relationships between these coefficients, establishing the second-order Mott relation and the Wiedemann-Franz law induced by disorder. This study develops a comprehensive theoretical framework elucidating the nonlinear thermoelectric transport mechanisms in quantum material systems.