Spin amplitude wave due to dipole-quadrupole hybridization in pseudospin-1 pyrochlore magnets
Phys. Rev. B 112, 054401 – Published 1 August, 2025
DOI: https://doi.org/10.1103/lg4b-152s
Abstract
We explore the quantum pseudospin-1 pyrochlore magnet featuring -based spinel oxides that addresses the formation of amplitude-modulated spin-density waves. We propose that the relatively small spin-orbit coupling and the small extra crystal field splitting in these materials create anisotropic exchange interactions and strong single-ion anisotropy, respectively, whose interplay becomes the source of quadrupolar moments selectively appearing on certain sublattices, leading to a spatially modulated hybrid of dipolar and quadrupolar moments. This mechanism represents the possibility of insulating magnets to form an exotic phase with coexisting liquid-solid properties.