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    Spin amplitude wave due to dipole-quadrupole hybridization in pseudospin-1 pyrochlore magnets

    Hiroki Nakai* and Chisa Hotta

    • *Contact author: nakai-hiroki3510@g.ecc.u-tokyo.ac.jp

    Phys. Rev. B 112, 054401 – Published 1 August, 2025

    DOI: https://doi.org/10.1103/lg4b-152s

    Abstract

    We explore the quantum pseudospin-1 pyrochlore magnet featuring Fe2+-based spinel oxides that addresses the formation of amplitude-modulated spin-density waves. We propose that the relatively small spin-orbit coupling and the small extra crystal field splitting in these materials create anisotropic exchange interactions and strong single-ion anisotropy, respectively, whose interplay becomes the source of quadrupolar moments selectively appearing on certain sublattices, leading to a spatially modulated hybrid of dipolar and quadrupolar moments. This mechanism represents the possibility of insulating magnets to form an exotic phase with coexisting liquid-solid properties.

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