Third-order optical response in -wave altermagnets: Analytical and numerical results from a microscopic model
Phys. Rev. B 114, 105128 – Published 18 August, 2026
DOI: https://doi.org/10.1103/l1hy-6njg
Abstract
Altermagnets represent a novel category of magnetic materials characterized by zero net magnetization yet featuring spin-split band structures, and they demonstrate distinctive orbital-spin locking phenomena. Commencing from the minimal multiorbital tight-binding Hamiltonian of -wave altermagnets, we conduct an analysis of the general formulas for the third-order injection and shift currents. These currents are solely determined by the quantum metric and quantum connection, and involve no Berry curvature contribution. In the ideal scenario where the -bond hopping approaches zero , we derive closed-form analytical solutions for the third-order photoconductivities. For the general situation with a finite value of , we present a perturbative analytical solution within the limit of , and this solution is verified through numerical calculations. Our research establishes a comprehensive theoretical description of the third-order optospintronic responses in -wave altermagnets based on a microscopic model. Moreover, it offers a viable approach for the experimental observation of pure quantum geometric effects.