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    Third-order optical response in d-wave altermagnets: Analytical and numerical results from a microscopic model

    Shihao Zhang*

    • *Contact author: zhangshh@hnu.edu.cn

    Phys. Rev. B 114, 105128 – Published 18 August, 2026

    DOI: https://doi.org/10.1103/l1hy-6njg

    Abstract

    Altermagnets represent a novel category of magnetic materials characterized by zero net magnetization yet featuring spin-split band structures, and they demonstrate distinctive orbital-spin locking phenomena. Commencing from the minimal multiorbital tight-binding Hamiltonian of d-wave altermagnets, we conduct an analysis of the general formulas for the third-order injection and shift currents. These currents are solely determined by the quantum metric and quantum connection, and involve no Berry curvature contribution. In the ideal scenario where the δ-bond hopping Vδ approaches zero (Vδ=0), we derive closed-form analytical solutions for the third-order photoconductivities. For the general situation with a finite value of Vδ, we present a perturbative analytical solution within the limit of Vδ≪Vπ, and this solution is verified through numerical calculations. Our research establishes a comprehensive theoretical description of the third-order optospintronic responses in d-wave altermagnets based on a microscopic model. Moreover, it offers a viable approach for the experimental observation of pure quantum geometric effects.

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