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    Controlled spin-to-charge conversion in noncollinear antiferromagnet-based Py/Mn3Pt heterostructures

    Indraneel Sinha1,*, Saurav Sachin1,*, Prashant Kumar2,†, Atul Pandey3, Bijoy Kumar Kuanr2, and Sujit Manna1,‡

    • *These authors contributed equally to this work.
    • †Present address: Motilal Nehru College, University of Delhi, South Campus, New Delhi 110021, India.
    • ‡Contact author: smanna@physics.iitd.ac.in

    Phys. Rev. B 112, 224428 – Published 16 December, 2025

    DOI: https://doi.org/10.1103/kpjb-6spp

    Abstract

    Noncollinear antiferromagnets (NCAFs) have recently emerged as promising candidates for future spintronic technologies, offering ultrafast switching, negligible stray fields allowing dense packing, and robustness against external magnetic perturbations. When interfaced with ferromagnets (FMs), they can strongly influence interfacial exchange and spin-torque mechanisms that enable manipulating magnetic order and realizing functionalities beyond conventional heavy metals (HMs) based FM/HM heterostructures. Here, we perform a broadband ferromagnetic resonance (FMR) study to systematically investigate the magnetization dynamics and spin-to-charge conversion in permalloy (Py) and Mn3Pt bilayers. High-quality Py films provide well-defined FMR spectra with a low Gilbert damping parameter (αeff≈9.8×10−3). We observe a pronounced enhancement of damping with intrinsic value αint≈3.1×10−2 in the Py/Mn3Pt bilayer, indicating efficient spin pumping into the NCAF layer. Frequency dependent linewidth analysis shows a predominantly Gilbert type damping in the bilayers and the corresponding effective spin-mixing conductance (geff↑↓≈4.8×1018m−2) is comparable to that of other high-performance antiferromagnetic heterostructures. These results are significant for establishing NCAFs as a candidate material for spin generation and highlight the potential of Py/Mn3Pt bilayers for efficient and ultrafast spintronic applications.

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