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Tunable roton-like exciton states via magnetic fields in two-dimensional layered systems
Phys. Rev. B 112, 195304 – Published 17 November, 2025
DOI: https://doi.org/10.1103/km2j-4qfp
Abstract
Excitons are charge neutral and thus weakly responsive to conventional gating, making magnetic fields a practical external control. Within an effective-mass framework that incorporates momentum-dependent sheet screening and field-induced center-of-mass/relative-motion couplings that is benchmarked against an analytic, constant- hydrogenic estimator, we compute dispersions and binding energies of intra- and interlayer excitons. Intralayer spectra are highly sensitive to screening yet display only weak quadratic diamagnetic shifts with negligible effective-mass renormalization. By contrast, interlayer spectra, which are less sensitive to modeling details, exhibit pronounced linear-in- energy shifts, enhanced binding, and substantial effective-mass increases. The finite spacer suppresses short-range screening, which smooths the interaction core and extends its long-range tail, thereby amplifying magnetic confinement. Consequently, low-lying interlayer excited states develop tunable roton-like minima for T, implying finite- brightening. The pronounced interlayer-intralayer contrast establishes magnetic fields as a selective knob for exciton-specific control and tunable optoelectronic functionality.