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Tunable roton-like exciton states via magnetic fields in two-dimensional layered systems

Yingda Chen1,2, Wen-Kai Lou2,*, and Kai Chang3,4,†

  • *Contact author: wklou@semi.ac.cn
  • †Contact author: kchang@zju.edu.cn

Phys. Rev. B 112, 195304 – Published 17 November, 2025

DOI: https://doi.org/10.1103/km2j-4qfp

Abstract

Excitons are charge neutral and thus weakly responsive to conventional gating, making magnetic fields a practical external control. Within an effective-mass framework that incorporates momentum-dependent sheet screening ε(q) and field-induced center-of-mass/relative-motion couplings that is benchmarked against an analytic, constant-εeff hydrogenic estimator, we compute dispersions and binding energies of intra- and interlayer excitons. Intralayer spectra are highly sensitive to screening yet display only weak quadratic diamagnetic shifts with negligible effective-mass renormalization. By contrast, interlayer spectra, which are less sensitive to modeling details, exhibit pronounced linear-in-B energy shifts, enhanced binding, and substantial effective-mass increases. The finite spacer D suppresses short-range screening, which smooths the interaction core and extends its long-range tail, thereby amplifying magnetic confinement. Consequently, low-lying interlayer excited states develop tunable roton-like minima for B≲30 T, implying finite-P brightening. The pronounced interlayer-intralayer contrast establishes magnetic fields as a selective knob for exciton-specific control and tunable optoelectronic functionality.

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