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    Complex magnetic transitions in the triangular net compound GdAl2Ge2

    Keke Feng1, Melissa G. Anderson2, Marcin Rosmus3, Alexandre Antezak3, Christopher Farago4, Emmanouil Frantzeskakis3, Franck Fortuna3, Andres F. Santander-Syro3, Gregory T. McCandless2 et al.

    Julia Y. Chan2 and Ryan E. Baumbach4

    Phys. Rev. B 113, 144430 – Published 21 April, 2026

    DOI: https://doi.org/10.1103/kjct-68sj

    Abstract

    Thermodynamic and electrical transport properties are reported for single crystals of the trigonal GdAl2Ge2, where complex antiferromagnetic ordering is seen at TN1 = 23.3 K and TN2 = 20.8 K and a rich phase diagram is revealed under applied magnetic fields. Angle-resolved photoemission spectroscopy (ARPES) measurements provide insights into this behavior by revealing a threefold symmetric Fermi surface that reflects the trigonal space-group symmetry. This promotes competing long-range Ruderman-Kittel-Kasuya-Yosida (RKKY) interactions between localized magnetic moments and is associated with the appearance of fine tuned ordered states. This is accompanied by intrinsic null orbital angular momentum (L = 0 for trivalent Gd), which yields Heisenberg spins and ensures that the symmetry of the Fermi surface dominates the magnetic behavior over wide temperature ranges. Comparisons are made to related triangular-net f-electron materials, providing guidance for understanding their diverse behaviors.

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