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EuAuSb: An odd-parity helical variation of altermagnetism

J. Sears1,*, Juntao Yao1,2, Zhixiang Hu2, Wei Tian3, Niraj Aryal1, Weiguo Yin1, A. M. Tsvelik1, I. A. Zaliznyak1, Qiang Li1,4 et al.

J. M. Tranquada1,†

  • *Contact author: jsears@bnl.gov
  • †Contact author: jtran@bnl.gov

Phys. Rev. B 112, 094455 – Published 26 September, 2025

DOI: https://doi.org/10.1103/k376-4cxw

Abstract

EuAuSb is a triangular-lattice Dirac semimetal in which a topological Hall effect has been observed to develop in association with a magnetically ordered phase. Our single-crystal neutron diffraction measurements have identified an incommensurate helical order in which individual ferromagnetic Eu2+ layers rotate in-plane by ∼120∘ from one layer to the next. An in-plane magnetic field distorts the incommensurate order, eventually leading to a first order transition to a state that is approximately commensurate and that is continuously polarized as the bulk magnetization approaches saturation. From an analysis of the magnetic diffraction intensities versus field, we find evidence for a dip in the ordered in-plane moment at the same field where the topological Hall effect is a maximum, and we propose that this is due to field-induced quantum spin fluctuations. Our electronic structure calculations yield exchange constants compatible with the helical order and show that the bands near the Fermi level lose their spin degeneracy via a mechanism similar to that in the collinear altermagnets. We find that, unlike the even symmetry seen in the altermagnets, the spin splitting in EuAuSb has odd-wave symmetry similar to that recently found in a number of coplanar magnetic materials.

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