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Complete superconducting phase diagram and flux pinning mechanisms in the yttrium-containing high-entropy alloy YNbTiZrHf

Rafał Idczak1, Wojciech Nowak1,2,*, and Adam Pikul2

  • *Contact author: wojciech.nowak@uwr.edu.pl

Phys. Rev. B 114, 094507 – Published 11 August, 2026

DOI: https://doi.org/10.1103/k1yr-t59z

Abstract

We report on the synthesis and characterization of an yttrium-containing high-entropy alloy (HEA) superconductor obtained from a nominal YNbTiZrHf composition. Structural analysis reveals a body-centered-cubic matrix with minor yttrium-rich hexagonal precipitates. Comprehensive measurements of electrical resistivity, magnetization, ac magnetic susceptibility, and specific heat confirm bulk type-II superconductivity with a transition temperature Tc≈6.1K, a critical current density Jc≈45kA/cm2, and an upper critical field μ0Hc2=12.5T, exceeding the Pauli limit due to strong spin-orbit scattering. The superconducting phase diagram, constructed from Jc(T), Jc(μ0H), and μ0H(T) data, is reported for a HEA superconductor. Flux pinning analysis indicates dominant surface pinning with a secondary point contribution, while collective pinning theory reveals a crossover from δTc-type to δl-type pinning with increasing field. The estimated depairing current density Jd≈21MA/cm2, which is more than 2 orders of magnitude higher than the experimental Jc, suggests significant potential for performance enhancement through microstructural optimization.

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