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    Mode-dependent emission thresholds and frequencies in metal nanoparticles within gain-enhanced media

    Karen Caicedo1,2, Nicole Recalde1, Milena Mora1, Alonso Moreta1, Maria Antonia Iatì3, Onofrio M. Maragò3, Melissa Infusino1,3, and Alessandro Veltri1,3,*

    • *Contact author: aveltri@usfq.edu.ec

    Phys. Rev. B 112, 195412 – Published 5 November, 2025

    DOI: https://doi.org/10.1103/jpp3-p5dp

    Abstract

    We present a mode-resolved analysis of emission thresholds in metal nanoparticles embedded within an infinite gain medium, using Mie scattering theory as a rigorous framework. Focusing on the first three resonant modes, we identify the onset of emission by locating the complex zeros of the electric scattering coefficient an(ω), which serve as indicators of lasing conditions. Our hybrid numerical scheme—combining coarse bracketing and two-dimensional Newton refinement—enables precise determination of both the threshold gain G•nth and corresponding emission frequency ω•nth across varying particle radii. The results uncover strong size-dependent behavior, with higher-order modes in larger particles exhibiting significantly reduced threshold gain. These insights elucidate the modal dynamics underlying plasmonic nanolasing and provide design guidelines for active photonic systems leveraging gain-enhanced nanoparticles.

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