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    Triple-well ferroelectricity and a kagomelike Chern flat band in two-dimensional multiferroic CuVP2Se6

    Brian Anchico1, Jingyi Duan1,*, Haojie Sun1, Minjun Wang1, Mikhail Talanov2, and Wei Jiang1,3,†

    • *Contact author: duanjy0518@gmail.com
    • †Contact author: wjiang@bit.edu.cn

    Phys. Rev. B 114, 175135 – Published 25 September, 2026

    DOI: https://doi.org/10.1103/jkkw-5bzw

    Abstract

    Two-dimensional multiferroics that host nontrivial topological bands offer a rich platform for correlated and tunable quantum phenomena, yet such materials remain rare. Here, using first-principles calculations, we reveal that monolayer CuVP2Se6 unites a tunable triple-well ferroelectric transition with a spin-polarized Chern flat band. The ferroelectric and paraelectric phases are close in energy and can be reversibly switched by moderate strain or an electric field. During the transition, a kagomelike flat band emerges near the Fermi level, which we describe via a minimal three-orbital tight-binding model on a triangular lattice. Furthermore, the system exhibits sizable magnetic anisotropy and a magnetization-dependent Chern insulating state: The Chern number is C=±1 for out-of-plane magnetization but becomes trivial when the moments rotate in-plane. These findings establish CuVP2Se6 as a promising candidate for exploring electrically tunable flat-band correlations and topological magnetism in a multiferroic monolayer.

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