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    Ultrafast optical evidence of coexisting density waves in bilayer nickelate La3Ni2O7

    Qi-Yi Wu1,2,*, De-Yuan Hu3,*, Chen Zhang1, Mengwu Huo3, Hao Liu1, Bo Chen1, Ying Zhou1, Zhong-Tuo Fu1, Chun-Hui Lv1 et al.

    Zi-Jie Xu1, Hai-Long Deng1, H. Y. Liu4, Jun Liu2, Yu-Xia Duan1, Meng Wang3,†, and Jian-Qiao Meng1,‡

    • *These authors contributed equally to this work.
    • †Contact author: wangmeng5@mail.sysu.edu.cn
    • ‡Contact author: jqmeng@csu.edu.cn

    Phys. Rev. B 112, 235110 – Published 2 December, 2025

    DOI: https://doi.org/10.1103/j6hl-t2sh

    Abstract

    Utilizing ultrafast optical pump-probe spectroscopy, we investigate the coexistence and competition of electronic orders in the bilayer nickelate La3Ni2O7. Our results reveal two coexisting density waves that can be selectively manipulated with light. We directly identify a spin-density wave (SDW) with electronic nematicity emerging below TSDW ≈140 K by measuring its spin dynamics, and discover a distinct, nonmagnetic charge order appearing below TDW ≈115 K. The central finding is the demonstration of differential optical control: the charge order is fragile, completely suppressed by a pump fluence of approximately 40 µJ/cm2, while the SDW is remarkably robust, persisting to 200 µJ/cm2. This work establishes a clear hierarchy in the stability of competing electronic orders and provides a powerful method for disentangling their interplay in quantum materials.

    Physics Subject Headings (PhySH)

    Corrections

    6 January, 2026

    Correction: Typographical errors in the label on the right vertical axis of the top panel of Fig. 4 and in the caption have been fixed.

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