High-field crossover from linear to nonlinear magnetoelectric effect in
Phys. Rev. B 114, 024417 – Published 20 July, 2026
DOI: https://doi.org/10.1103/j66k-pc7d
Abstract
The -site magnetic spinel exhibits a simple Néel-type collinear antiferromagnetic ordering below K, accompanied by a strong linear magnetoelectric effect. Here, we report magnetization and electric polarization measurements on single crystals of up to high magnetic fields. We show that the magnetoelectric polarization undergoes a crossover from linear to nonlinear behavior with increasing magnetic field, followed by complete suppression upon reaching the field-polarized ferromagnetic state, where inversion symmetry is recovered. Our microscopic spin model, reproducing the observed field evolution of the magnetoelectric response, evidences weak anisotropy that is crucial for the effective magnetoelectric control of the antiferromagnetic state [Phys. Rev. Lett. 135, 126704 (2025)].