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Absence of critical fluctuations at the bandwidth-controlled Mott transition in a molecular conductor

Tim Thyzel1, Lars Franke2, Markus Garst2,3, Harald Schubert1, Michael Lang1, Takahiko Sasaki4, and Jens Müller1,*

  • *Contact author: j.mueller@physik.uni-frankfurt.de

Phys. Rev. B 112, L121101 – Published 2 September, 2025

DOI: https://doi.org/10.1103/j1jp-yy68

Abstract

The universality class of the Mott metal-insulator transition in electronic systems strongly coupled to the lattice degrees of freedom has been the subject of recent debate. While transport scaling exponents as well as a critical slowing down of resistance fluctuations point towards Ising-type criticality, a strong involvement of the lattice elasticity suggests a mean-field scenario instead. We investigate the low-frequency resistance noise in the model system κ−(ET)2Cu[N(CN)2]Cl(κ−Cl)—selected because it is known to exhibit critical elasticity—tuned to the Mott end point by hydrostatic pressure. Contrary to previous reports for the related, deuterated κ-Br compound, we do not find any indication of a critical slowing down, but observe a strong and anisotropic change of the relative resistance noise level in the metallic compared to the insulating phase. We speculate within the framework of isostructural criticality that a critical slowing down might emerge in the presence of structural disorder.

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