Enhancement of the superconducting transition temperature due to multiband effect in the topological nodal-line semimetal
Phys. Rev. B 112, 054504 – Published 6 August, 2025
DOI: https://doi.org/10.1103/hsdq-2tp9
Abstract
We report a systematic study of the normal-state and superconducting properties of single-crystal . Sn doping enhances the superconducting temperature up to 5.1 K while also significantly increasing impurity scattering in the crystals. For and 0.018, the specific-heat jump at exceeds the Bardeen-Cooper-Schrieffer (BCS) weak-coupling value of 1.43, indicating the realization of strong-coupling superconductivity in undoped and slightly-Sn-doped . Substituting Pb with more Sn lowers the specific-heat jump at below the BCS value of 1.43, which cannot be explained by a single-gap model. Rather, the observed specific-heat data of moderately-Sn-doped are reproduced by a two-gap model. Our density functional theory calculations suggest that three-dimensional Fermi pockets appear due to a reduction of the spin-orbit gap with Sn doping, and the multiband effect arising from these emergent Fermi pockets enhances the effective electron-phonon coupling strength, leading to the increase in of .