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Quantum oscillation fingerprints of altermagnetism in hole-doped RuO2

Yuchi Yang and Yusheng Hou*

  • Guangdong Provincial Key Laboratory of Magnetoelectric Physics and Devices, Institute of Neutron Science and Technology, School of Physics, Sun Yat-Sen University, Guangzhou 510275, China

  • *Contact author: houysh@mail.sysu.edu.cn

Phys. Rev. B 114, 094410 – Published 6 August, 2026

DOI: https://doi.org/10.1103/h8sf-h9nw

Abstract

Altermagnetism, characterized by its ferromagnetism-like spin-splitting band structure and antiferromagnetism-like magnetic order, has garnered considerable attention recently. Although hole doping may promote magnetism in the debated altermagnet (AM) candidate RuO2, the evolution of its electronic and magnetic properties under hole doping remains poorly understood. Based on first-principles calculations, we employ quantum oscillations to study hole-doped RuO2. We find that hole doping can enhance spin splitting and reconstruct the Fermi surface in RuO2, which is revealed by the angle-dependent quantum oscillation frequency. By tracking a pair of closed Fermi-surface pockets, we identify a meaningful correlation between the magnetic moment of Ru and a quantum-oscillation-based signature of spin splitting. This correlation follows a quasilinear trend over a broad doping range, which can be captured by a minimal two-dimensional d-wave AM model. In addition, the hole-doped RuO2 exhibits a transition from a nonmagnetic to an AM state via an intermediate state. The quasilinear correlation through quantum oscillation and the distinct quantum oscillation frequency of the stable AM state can serve as useful signatures for identifying the AM state in RuO2. Our results provide a comprehensive framework for understanding hole-doped RuO2, offering insights into AM transitions and their identification.

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