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    Optospintronic effects in an A-type antiferromagnetic Ti2C MXene spin valve

    You Zhou1, Jiahui Wang1, Haoshen Ye2, Dingwen Zhang3, Leiming Chen1, and Jianli Wang1,*

    • *Contact author: jlwang@cumt.edu.cn

    Phys. Rev. B 112, 125430 – Published 30 September, 2025

    DOI: https://doi.org/10.1103/gw8k-trxk

    Abstract

    The self-spin valve, an important giant-magnetoresistance effect observed down to a monolayer thickness, is highly desirable because of the ease of experimental sample preparation. Here, we target the A-type antiferromagnetic Ti2C monolayer MXene. Our first-principles calculations based on the density functional theory demonstrate that biaxial strain in the xy plane is an effective approach to achieve the transition from an antiferromagnetic semiconductor to a room-temperature ferromagnetic metal in the A-type antiferromagnetic Ti2C monolayer MXene. The out-of-plane easy magnetization axis is robust under the strain. Interestingly, a nonzero magneto-optical Kerr effect signal emerges with a peak Kerr angle of 0.06 rad under a 7% tensile strain. Our results indicate that strain can effectively modulate the optospintronic valve.

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