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    Electrical switching of multiple and layer-dependent topological spin textures by interlayer polarization coupling

    Jingbiao Yuan1, Xiong-Xiong Xue1,*, Yee Sin Ang2, Ke-Qiu Chen3, and Li-Ming Tang3

    • *Contact author: xxxue@hnu.edu.cn

    Phys. Rev. B 114, 084413 – Published 14 August, 2026

    DOI: https://doi.org/10.1103/grzb-lr1k

    Abstract

    Based on first-principles calculations and atomistic simulations, this work reveals the underlying mechanism of interlayer polarization coupling in governing topological spin states. We demonstrated polarization-guided Dzyaloshinskii-Moriya interaction sign reversal in the predicted multiferroic material Cr2Sn2Te6, interlayer polarization coupling mediated the multiple modulation of spin textures in the Cr2Sn2Te6/In2Se2 heterostructure, and the layer-dependent topological Hall effect in the Cr2Sn2Te6/In2Se3/Cr2Sn2Te6 sandwich structure. Combined with magnetic field control and ferroelectric polarization, the stable and flexible switching between various types of skyrmions can be achieved in Cr2Sn2Te6. In the Cr2Sn2Te6/In2Se3 heterostructure, the synergistic interaction between interlayer polarization coupling and strain effectively modulates the Dzyaloshinskii-Moriya interaction strength and magnetic anisotropy, enabling continuous and reversible transitions between multiple spin textures, including skyrmions, bimerons, in-plane ferromagnetic states, and out-of-plane ferromagnetic states. The Cr2Sn2Te6/In2Se3/Cr2Sn2Te6 integrates two polarization coupling modes within a single system, establishing a multitopological coupling platform in the vertical dimension. By regulating ferroelectric polarization reversal, directional transfer of spin textures and their topological Hall signals between different layers is achievable, enabling nonvolatile electrical control of the layer-dependent topological Hall effect.

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