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    Field-induced evolution of the ferrimagnetic ground state and possible thermally induced spin chirality in Tb3Ru4Al12

    Kosuke Karube1,*, Shang Gao1,2, Nguyen Duy Khanh1,3, Akiko Kikkawa1, Hironori Nakao4, Hajime Sagayama4, Max Hirschberger1,3, Taro Nakajima1,5, Taka-hisa Arima1,6 et al.

    Masahito Mochizuki7, Yoshinori Tokura1,3,8, and Yasujiro Taguchi1,9,†

    • *Contact author: kosuke.karube@riken.jp
    • †Contact author: y-taguchi@riken.jp

    Phys. Rev. B 113, 134417 – Published 10 April, 2026

    DOI: https://doi.org/10.1103/gdls-q39l

    Abstract

    Magnetic frustration in kagomé lattice materials has attracted considerable attention as a source of novel magnetic properties and magnetotransport phenomena. Here we report experimental evidence for collinear ferrimagnetic ordering and multiple field-induced magnetic transitions in Tb3Ru4Al12 with a breathing kagomé lattice, revealed by field-dependent resonant x-ray scattering measurements performed at 8 K. The Hall response shows significant deviation from the conventional behavior above the ordering temperature, which can be plausibly interpreted in terms of thermally induced scalar spin chirality. Theoretical calculations reveal the emergence of net scalar spin chirality, whose magnitude depends on Ising-type magnetic anisotropy, in good agreement with experimental results on breathing kagomé magnets with different magnitude of the easy-axis anisotropy. This study highlights that nontrivial magnetotransport phenomena in breathing kagomé magnets may arise from thermally fluctuating spin moments with finite scalar spin chirality, even when the ground state is a collinear ferrimagnet.

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