Propagation of short pulses in Rydberg exciton medium under blockade conditions
Phys. Rev. B 113, 245307 – Published 22 June, 2026
DOI: https://doi.org/10.1103/gd71-59k8
Abstract
Propagation of short pulses through crystal containing Rydberg excitons is studied with the use of the density matrix formalism and the finite difference time domain method. Effects of the so-called Rydberg blockade are studied extensively, exploring not only a reduction of absorption (bleaching) but also power-dependent changes of dispersive properties of the medium. The role of an exciton lifetime and coherent population oscillations in the dynamics of the system are investigated. A pump-probe setup with two pulses is also studied, showing a good agreement with recent experimental results. Calculations are performed for Rydberg states, both for low and high principal quantum numbers.