Temperature-dependent ultrafast carrier and lattice dynamics in Dirac semimetals and
Phys. Rev. B 111, 245304 – Published 24 June, 2025
DOI: https://doi.org/10.1103/g2lh-1nb6
Abstract
This study examines the ultrafast carrier dynamics of topological semimetals and , highlighting the influence of their distinct electronic structures. Transient absorption spectroscopy in reflectance mode reveals that exhibits a sharp feature at 2.03 eV, linked to Dirac states near the Fermi level, while shows a broader, featureless response due to its Dirac states lying 0.5 eV below the Fermi level. In the near-infrared region, demonstrates rapid state filling and short-lived dynamics, whereas supports prolonged absorption due to accessible Dirac states. Temperature-dependent studies reveal a nonmonotonic relaxation in , attributed to a Lifshitz transition around T*≈ 50 K, altering the Fermi surface topology. In contrast, exhibits conventional relaxation dynamics across temperatures. These findings underscore the role of Dirac states and topological transitions in shaping carrier dynamics, offering insights for advancing optoelectronic and thermal management technologies.