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    Temperature-dependent ultrafast carrier and lattice dynamics in Dirac semimetals NiTe2 and PdTe2

    Prince Sharma1,2,*, Saurabh K. Saini1,2, Kapil Kumar1,2, and Mahesh Kumar1,2,3,†

    • *Contact author: sharmapvats8@gmail.com
    • †Contact author: mkumar@csir.res.in

    Phys. Rev. B 111, 245304 – Published 24 June, 2025

    DOI: https://doi.org/10.1103/g2lh-1nb6

    Abstract

    This study examines the ultrafast carrier dynamics of topological semimetals NiTe2 and PdTe2, highlighting the influence of their distinct electronic structures. Transient absorption spectroscopy in reflectance mode reveals that NiTe2 exhibits a sharp feature at 2.03 eV, linked to Dirac states near the Fermi level, while PdTe2 shows a broader, featureless response due to its Dirac states lying 0.5 eV below the Fermi level. In the near-infrared region, NiTe2 demonstrates rapid state filling and short-lived dynamics, whereas PdTe2 supports prolonged absorption due to accessible Dirac states. Temperature-dependent studies reveal a nonmonotonic relaxation in NiTe2, attributed to a Lifshitz transition around T*≈ 50 K, altering the Fermi surface topology. In contrast, PdTe2 exhibits conventional relaxation dynamics across temperatures. These findings underscore the role of Dirac states and topological transitions in shaping carrier dynamics, offering insights for advancing optoelectronic and thermal management technologies.

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