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    Out-of-plane spin polarization due to spin-orbit torque effects in single-layer epitaxial La0.67Sr0.33MnO3 films

    Yifei Wang1, Wending Liu1, Zhirui Wang1, Zhiqiang Zhang1, Teng Gao1, Zhenlin Jia1, Xiaoyu Feng1,2, Jiguang Yao1,3, Hai Xu4,5 et al.

    Bin Wang4,5, Dangwei Guo1, Desheng Xue1, Mingsu Si6, and Xiaolong Fan1,*

    • *Contact author: fanxiaolong@lzu.edu.cn

    Phys. Rev. B 114, 084403 – Published 3 August, 2026

    DOI: https://doi.org/10.1103/fzk1-yrhz

    Abstract

    We investigate spin-orbit torque effects in epitaxial La0.67Sr0.33MnO3 (LSMO) films via spin-torque ferromagnetic resonance. In the absence of any extrinsic spin source, spin currents with σy, σz, and σx polarizations are observed in a single LSMO layer. Decomposing the response within the Kubo linear response formalism reveals that the σy component is composed of both interband and intraband terms, whereas the σz and σx components are dominated by the interband term. The interband contribution is closely linked to the thickness-dependent strain and Mn-eg level splitting. This effect is attributed to a redistribution of the spin Berry curvature, induced by a structural gradient of octahedral distortions and rotations that breaks inversion symmetry. In contrast, the intraband contribution is attributed to a Rashba-like response in the inversion-symmetry-broken regions. These results indicate that octahedral distortions and rotations in epitaxial LSMO can reshape the Mn-eg band structure and interband transitions, thereby modifying the intrinsic spin-transport tensor and making the spin polarization components sensitive to structural details. Our work establishes a link between structural distortion and spin current generation in epitaxial LSMO films and provides a basis for designing field-free magnetization switching in single-layer oxide spintronic devices.

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