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Ising spin ladders of orthopyroxene CoGeO3

Pavel A. Maksimov1,2, Andrey F. Gubkin2, Alexey V. Ushakov2, Alexander I. Kolesnikov3, Matthew S. Cook4, Michael A. McGuire4, Günther J. Redhammer5, Andrey Podlesnyak3, and Sergey V. Streltsov2,*

  • *Contact author: streltsov.s@gmail.com

Phys. Rev. B 112, L220407 – Published 10 December, 2025

DOI: https://doi.org/10.1103/fxrl-yr9g

Abstract

We present thermodynamic and spectroscopic measurements for an orthopyroxene CoGeO3 with magnetic Co2+ ions that form quasi-one-dimensional ladders. We show that noncollinear magnetic order below TN=32 K can be stabilized by a strong local easy-axis anisotropy of jeff=1/2 moments, which is induced by ligand octahedra distortions. Extraction of a magnetic Hamiltonian from inelastic neutron scattering measurements supports this interpretation and allows us to establish an effective magnetic model. The resulting exchange Hamiltonian justifies CoGeO3 as a realization of an Ising spin ladder compound.

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