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Effect of uniaxial stress on helimagnetic phases in the square-lattice itinerant magnet EuAl4

Masaki Gen1,2,*, Takuya Nomoto3, Hiraku Saito1, Taro Nakajima1,2,4, Yusuke Tokunaga5, Rina Takagi1, Shinichiro Seki6,7, and Taka-hisa Arima2,5

  • *Contact author: gen@issp.u-tokyo.ac.jp

Phys. Rev. B 113, L100406 – Published 11 March, 2026

DOI: https://doi.org/10.1103/frqw-vng9

Abstract

We investigate uniaxial-stress effects on the magnetic phase diagram of the square-lattice itinerant magnet EuAl4, where strong coupling among spin, lattice, and charge produces a variety of helimagnetic phases, including rhombic and square skyrmion lattices. Combining resistivity and magnetization measurements with neutron scattering, we find that compressive stresses of only several tens of megapascal along [010] enhance antiferromagnetic character and shorten the magnetic modulation period in the lowest-temperature single-Q spiral state, thereby driving the critical temperatures and fields of multiple phases to higher values. First-principles calculations show that increasing orthorhombic lattice distortion deforms the Fermi surface relevant to the magnetism, providing compelling evidence that Fermi-surface nesting plays a crucial role in stabilizing the helical magnetic modulations in EuAl4.

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