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    Emergent room-temperature anomalous and topological Hall responses in the epitaxial ferromagnetic Weyl nodal-line metal Fe5Si3

    Shubhashish Pati1, Sonali Srotaswini Pradhan2, Abhay Pandey1, Nikita Sharma1, Nanhe Kumar Gupta1,*, Nakul Kumar1, Soumyarup Hait1,†, Nidhi Shukla1, Saurav Singh1 et al.

    Vidhi Jain1, Mitali1, V. Kanchana2,‡, and Sujeet Chaudhary1,§

    • *Present address: Centre for Magnetic and Spintronic Materials (CMSM), National Institute for Materials Science (NIMS), 1-2-1 Sengen, Tsukuba, Ibaraki 305-0047, Japan.
    • †Present address: School of Physics and Astronomy, University of Leeds, Leeds LS2 9JT, United Kingdom.
    • ‡Contact author: kanchana@phy.iith.ac.in
    • §Contact author: sujeetc@physics.iitd.ac.in

    Phys. Rev. B 114, 094426 – Published 20 August, 2026

    DOI: https://doi.org/10.1103/flxb-4ktc

    Abstract

    The interplay between real and reciprocal space topology yields intrinsically linked transport phenomena in topological magnetic material systems. In particular, broken time-reversal symmetry together with strong Dzyaloshinskii-Moriya interaction and pronounced uniaxial anisotropy can simultaneously stabilize momentum-space Berry-curvature singularities (Weyl nodes) and real-space chiral spin textures. The concurrent realization of these dual topological features remains exceptionally rare, particularly in epitaxial thin films. Here, we present a combined first-principles and detailed magnetotransport investigation of epitaxial Fe5Si3 thin films, establishing the material as a magnetic Weyl nodal-line metal in which density functional theory (DFT) calculations uncover a topologically nontrivial electronic structure featuring six pairs of Weyl nodes near the Fermi level (EF) and pronounced Berry-curvature hot spots at high-symmetry points, and accompanied by a large topological Hall response. High-quality epitaxial films exhibit robust ferromagnetism with a high Curie temperature (TC) of approximately 370 K and strong magnetocrystalline anisotropy. The magnetotransport measurements on epitaxial films reveal the corresponding Berry-curvature-driven responses, including a significantly large intrinsic anomalous Hall conductivity of 504 S/cm and a high anomalous Hall angle of 5.5%, which is in good agreement with DFT calculations. Furthermore, a substantial topological Hall resistivity of 1.6μΩcm is robust across a wide temperature range, indicating the possibility of robust chiral spin textures in the thin-film geometry. These combined theoretical and experimental results establish Fe5Si3 as a unique, low-cost, centrosymmetric magnetic Weyl nodal-line material, providing a versatile platform for exploring coupled real- and reciprocal-space topologies in topological spintronic applications.

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