Emergent room-temperature anomalous and topological Hall responses in the epitaxial ferromagnetic Weyl nodal-line metal
Phys. Rev. B 114, 094426 – Published 20 August, 2026
DOI: https://doi.org/10.1103/flxb-4ktc
Abstract
The interplay between real and reciprocal space topology yields intrinsically linked transport phenomena in topological magnetic material systems. In particular, broken time-reversal symmetry together with strong Dzyaloshinskii-Moriya interaction and pronounced uniaxial anisotropy can simultaneously stabilize momentum-space Berry-curvature singularities (Weyl nodes) and real-space chiral spin textures. The concurrent realization of these dual topological features remains exceptionally rare, particularly in epitaxial thin films. Here, we present a combined first-principles and detailed magnetotransport investigation of epitaxial thin films, establishing the material as a magnetic Weyl nodal-line metal in which density functional theory (DFT) calculations uncover a topologically nontrivial electronic structure featuring six pairs of Weyl nodes near the Fermi level () and pronounced Berry-curvature hot spots at high-symmetry points, and accompanied by a large topological Hall response. High-quality epitaxial films exhibit robust ferromagnetism with a high Curie temperature () of approximately 370 K and strong magnetocrystalline anisotropy. The magnetotransport measurements on epitaxial films reveal the corresponding Berry-curvature-driven responses, including a significantly large intrinsic anomalous Hall conductivity of 504 S/cm and a high anomalous Hall angle of 5.5%, which is in good agreement with DFT calculations. Furthermore, a substantial topological Hall resistivity of is robust across a wide temperature range, indicating the possibility of robust chiral spin textures in the thin-film geometry. These combined theoretical and experimental results establish as a unique, low-cost, centrosymmetric magnetic Weyl nodal-line material, providing a versatile platform for exploring coupled real- and reciprocal-space topologies in topological spintronic applications.