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    Influence of magnon-magnon and magnon-phonon interactions on magnon relaxation under external strain and magnetic fields in monolayer MnSe2

    Chang-Hao Ding1, Wenwen Liu1, Yuan Yao1, Hao Chen1, Nannan Luo1, Jiang Zeng1, Li-Ming Tang1, Hui Pan2,*, and Ke-Qiu Chen1,†

    • *Contact author: panhui@nus.edu.sg
    • †Contact author: keqiuchen@hnu.edu.cn

    Phys. Rev. B 113, 115403 – Published 3 March, 2026

    DOI: https://doi.org/10.1103/fhqs-mvfw

    Abstract

    Understanding and controlling magnon relaxation in two-dimensional (2D) ferromagnets is crucial for applications in spintronics, as it governs magnon-based spin transport and device performance. However, existing studies have been largely confined to systems with low Curie temperatures, leaving near-room-temperature 2D ferromagnets rarely explored. Here, we combine spin-wave theory with first-principles calculations to investigate magnon relaxation in the room-temperature 2D ferromagnet MnSe2, considering both magnon-magnon interactions (MMIs) and magnon-phonon interactions (MPIs) and analyzing their effects under external strain and magnetic fields. We find that a MPI exhibits a strong, nonmonotonic strain dependence due to its coupling to lattice distortions, whereas a MMI is primarily controlled by magnetic fields and is insensitive to strain. At room temperature, a MMI dominates the relaxation process, while the dominant mechanism can be largely reversed by strain and magnetic fields, especially at low temperatures and large wave vectors. These findings highlight the complementary roles of MPIs and MMIs in MnSe2, offering potential strategies for tailoring magnon relaxation in magnon-based spintronic devices.

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