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    Evolution of pairing symmetry in FeSe1−xSx as probed by in-plane strain tuning of Tc

    Ruixian Liu*,†, Qi Tang*, Chang Liu, Wenting Zhang, Chunyi Li, Kaijuan Zhou, Qiaoyu Wang, and Xingye Lu‡

    • Center for Advanced Quantum Studies, School of Physics and Astronomy, Beijing Normal University, Beijing, 100875, China and Key Laboratory of Multiscale Spin Physics, Ministry of Education, Beijing 100875, China

    • *These authors contributed equally to this work.
    • †Contact author: liurx@mail.bnu.edu.cn
    • ‡Contact author: luxy@bnu.edu.cn

    Phys. Rev. B 112, 094514 – Published 18 September, 2025

    DOI: https://doi.org/10.1103/f6jb-yvyj

    Abstract

    In iron-based superconductors (FeSCs), the interplay between electronic nematicity and superconductivity is essential for understanding the exotic superconducting ground state. In the nematic regime, in-plane strain (ɛ) tuning of the superconducting transition temperature Tc [ΔTc(ɛ)=αɛ+βɛ2] offers a unique approach to investigate the evolution of pairing symmetry if both s- and d-wave pairing instabilities are relevant. Here, we employ in-plane strain to tune the Tc of FeSe1−xSx, in which both nematicity and superconductivity undergo significant changes with doping. While Tc is usually suppressed quadratically with ɛ in optimally doped BaFe2As2, ΔTc(ɛ) in FeSe1−xSx dominated by ΔTc(ɛ)=βɛ2 changes its sign from β < 0 in FeSe to β > 0 in FeSe1−xSx (x≳0.10), indicating an evolution of the pairing symmetry from an s± state toward an s+d wave state. These findings highlight the ΔTc(ɛ) as a powerful probe for elucidating the superconducting pairing symmetry in the nematic regime of FeSCs and provide unique insights into the evolution of pairing symmetry in FeSCs.

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