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    Toward a unified description of valley polarization in two-dimensional tetragonal altermagnets driven by strain and in-plane magnetization

    Bo Huang, Churen Gui, Ao Zhang, Zhixiong Yang, Shu-Zong Li, Zhenqing Li, Hongxing Li, and Wei-Bing Zhang*

    • *Contact author: zhangwb@csust.edu.cn

    Phys. Rev. B 114, 045421 – Published 16 July, 2026

    DOI: https://doi.org/10.1103/f58d-vqf9

    Abstract

    Altermagnetism provides a promising platform for valleytronics applications due to its symmetry-protected spin-valley locking. While uniaxial strain and in-plane magnetization have recently emerged as novel routes to induce valley polarization in altermagnets, a unified theoretical framework elucidating their microscopic mechanisms remains absent. Here, we use a tight-binding (TB) model to show that both uniaxial strain and in-plane magnetization can induce valley polarization in two-dimensional (2D) tetragonal altermagnets by breaking the C4zT symmetry, although driven by distinct mechanisms. Specifically, uniaxial strain tunes valley polarization by modulating anisotropic hopping, yielding a monotonic dependence whose sign can be reversed by switching the strain axis (x/y) or type (compressive/tensile). In contrast, in-plane magnetization generates valley polarization via weak ferromagnetism, exhibiting a characteristic cos2ϕ dependence determined by the spin direction. Crucially, these model predictions are confirmed by first-principles calculations on a d-wave altermagnet monolayer Mo2Te2O, demonstrating tunable valley polarization. Our findings establish a unified theoretical framework for the control of valley polarization in 2D tetragonal altermagnets, providing a foundation for the development of valleytronics.

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