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    RKKY signatures as a probe for intrinsic magnetism and differentiation between axion insulator and quantum anomalous Hall phases in MnBi2Te4 films

    Ya-Xi Li, Zi-Jian Chen, Rui-Qiang Wang, Ming-Xun Deng, Mou Yang, and Hou-Jian Duan*

    • Guangdong Basic Research Center of Excellence for Structure and Fundamental Interactions of Matter, Guangdong Provincial Key Laboratory of Quantum Engineering and Quantum Materials, School of Physics, South China Normal University, Guangzhou 510006, China and Guangdong-Hong Kong Joint Laboratory of Quantum Matter, Frontier Research Institute for Physics, South China Normal University, Guangzhou 510006, China

    • *Contact author: dhjphd@163.com

    Phys. Rev. B 113, 155148 – Published 24 April, 2026

    DOI: https://doi.org/10.1103/f4pr-r83b

    Abstract

    We present a systematic study of the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction in MnBi2Te4 films under both dark and illuminated conditions. In the dark, the intrinsic magnetism of MnBi2Te4 is shown to yield a stronger anisotropic RKKY spin model compared to nonmagnetic topological insulators, providing a clear signature for differentiating these systems. Furthermore, key band properties—such as energy gap, band degeneracy/splitting, and topological deformations of the Fermi surface—imprint distinct signatures on the RKKY interaction, enabling clear discrimination between axion insulators (AI) and quantum anomalous Hall (QAH) insulators in even- and odd-septuple-layer (SL) films. This discrimination manifests in multiple ways: through the Fermi-energy dependence or spatial oscillations of the interaction for impurities on the same surface, or via the presence versus absence of spin-frustrated terms for those on different surfaces. Under off-resonant circularly polarized light, additional phase-transition-related fingerprints also emerge to distinguish these two phases, such as sign reversals of spin-frustrated terms in even-SL films versus chirality-selective double-dip structures of collinear RKKY components in odd-SL films. Overall, this work establishes RKKY interactions as a sensitive magnetic probe for distinguishing between AI phase (even-SL) and QAH phase (odd-SL), thereby complementing conventional electrical measurements while providing new insights into the influence of intrinsic magnetism on the surface-state band structure.

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