Low-temperature magnetic structure and lattice response in
Phys. Rev. B 113, 064403 – Published 3 February, 2026
DOI: https://doi.org/10.1103/dxw2-4fvl
Abstract
We investigated the structural and magnetic properties of single-crystalline using high-resolution synchrotron x-ray diffraction and x-ray resonant magnetic scattering (XRMS) at the Sm and edges. Temperature-dependent diffraction measurements confirm that maintains its tetragonal symmetry from room temperature down to 8 K, with lattice parameters showing anomalous behavior below the resistivity minimum (). Notably, the c-axis lattice parameter exhibits a plateau and subsequent increase near the Néel temperature, indicating magnetoelastic coupling. XRMS measurements reveal a commensurate antiferromagnetic structure with a propagation vector . Our measurement shows that the Sm moments are aligned within the plane and arranged in a stacking along the axis. Comparison with related compounds (RE = Pr, Nd, and Gd) suggests that in-plane moment orientation and associated magnetic frustration play a key role in the emergence of the resistivity minimum. Differences in spin-orbit and magnetoelastic coupling across the series highlight their importance in governing low-temperature transport behavior.