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    Low-temperature magnetic structure and lattice response in SmCuAs2

    M. G. Kim1,*, C. Neupane1, Y. Yu1, R. Acevedo-Esteves2, C. Nelson2, D. Evans3, E. D. Mun3, D. F. Agterberg1, and J.-W. Kim4

    • *Contact author: mgkim@uwm.edu

    Phys. Rev. B 113, 064403 – Published 3 February, 2026

    DOI: https://doi.org/10.1103/dxw2-4fvl

    Abstract

    We investigated the structural and magnetic properties of single-crystalline SmCuAs2 using high-resolution synchrotron x-ray diffraction and x-ray resonant magnetic scattering (XRMS) at the Sm L2 and L3 edges. Temperature-dependent diffraction measurements confirm that SmCuAs2 maintains its tetragonal symmetry from room temperature down to 8 K, with lattice parameters showing anomalous behavior below the resistivity minimum (T≈30K). Notably, the c-axis lattice parameter exhibits a plateau and subsequent increase near the Néel temperature, indicating magnetoelastic coupling. XRMS measurements reveal a commensurate antiferromagnetic structure with a propagation vector q=(0,0,0.5). Our measurement shows that the Sm moments are aligned within the ab plane and arranged in a ++−− stacking along the c axis. Comparison with related RECuAs2 compounds (RE = Pr, Nd, and Gd) suggests that in-plane moment orientation and associated magnetic frustration play a key role in the emergence of the resistivity minimum. Differences in spin-orbit and magnetoelastic coupling across the series highlight their importance in governing low-temperature transport behavior.

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