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    Multiple magnetic transitions, metamagnetism, and topological Hall effect in the rare-earth based plumbide GdRhPb

    Rajesh Swami1, Sonali S Pradhan2, V. Kanchana2,*, and Z. Hossain1,†

    • *Contact author: kanchana@phy.iith.ac.in
    • †Contact author: zakir@iitk.ac.in

    Phys. Rev. B 113, 035149 – Published 26 January, 2026

    DOI: https://doi.org/10.1103/dx66-ywt9

    Abstract

    We present a comprehensive investigation of the physical properties of a candidate nodal-line semimetal GdRhPb single crystals, through magnetization, heat capacity, and magnetotransport measurements. Temperature-dependent magnetization [χ(T)] along different crystallographic directions confirm that Gd ions are in the trivalent state and exhibit antiferromagnetic (AFM) ordering below TN1=17.6 K, followed by a second magnetic transition at TN2=15.3 K. Electrical resistivity measurement exhibits metallic behavior, followed by a sharp increase at just below TN1, indicative of AFM superzone gap formation. These AFM phase transitions are further corroborated by the temperature-dependent heat capacity. Within the AFM state, isothermal magnetization [M(H)] data reveal multiple field-induced metamagnetic (MM) transitions. Moreover, transverse and longitudinal magnetoresistance data show a sharp drop at critical fields, aligning with the MM transitions observed in M(H) data. Hall resistivity analysis in the paramagnetic region indicates a crossover from single carrier-dominated electrical transport to contributions from multiple carrier types. Interestingly, a distinct humplike anomaly in the Hall resistivity below TN1, not scaling with M(H), suggests the presence of the topological Hall contribution. Additionally, the constructed H−T phase diagram for H⊥c reveals at least four distinct magnetic phases, highlighting the compound's complex low-temperature magnetic behavior. Furthermore, first-principles calculations reveal that GdRhPb is a topologically nontrivial nodal-line semimetal, characterized by drumhead surface states and a nonzero Berry phase.

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