Disordered ground state in the three-dimensional face-centered frustrated spin- system
Phys. Rev. B 112, 054421 – Published 7 August, 2025
DOI: https://doi.org/10.1103/dmvp-xj68
Abstract
Frustrated magnetism in face-centered-cubic (fcc) magnetic sublattices remains underexplored but holds considerable potential for exotic magnetic behavior. Here we report on the crystal structure and the magnetic and thermodynamic properties of the -site-vacant hydroxide double perovskite . Despite dominant antiferromagnetic interactions among moments, evidenced by a negative Curie-Weiss temperature, the lack of a sharp thermodynamic transition down to 350 mK implies the absence of long-range magnetic order. However, a broad hump in the specific heat at 1.6 K suggests short-range correlations. Neutron diffraction at low temperatures confirms the presence of three-dimensional antiferromagnetic correlations, manifested as diffuse magnetic scattering with a correlation length and magnetic propagation vectors and at 20 mK.