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    Disordered ground state in the three-dimensional face-centered frustrated spin-52 system MnSn(OH)6

    Kaushick K. Parui1, Anton A. Kulbakov1, Ellen Häußler2, Nikolai S. Pavlovskii1, Aswathi Mannathanath Chakkingal1, Maxim Avdeev3,4, Roman Gumeniuk5, Sergey Granovsky1, Alexander Mistonov1 et al.

    Sergei A. Zvyagin6, Thomas Doert2, Dmytro S. Inosov1,7,*, and Darren C. Peets1,†

    • *Contact author: dmytro.inosov@tu-dresden.de
    • †Contact author: darren.peets@tu-dresden.de

    Phys. Rev. B 112, 054421 – Published 7 August, 2025

    DOI: https://doi.org/10.1103/dmvp-xj68

    Abstract

    Frustrated magnetism in face-centered-cubic (fcc) magnetic sublattices remains underexplored but holds considerable potential for exotic magnetic behavior. Here we report on the crystal structure and the magnetic and thermodynamic properties of the A-site-vacant hydroxide double perovskite MnSn(OH)6. Despite dominant antiferromagnetic interactions among Mn2+ moments, evidenced by a negative Curie-Weiss temperature, the lack of a sharp thermodynamic transition down to 350 mK implies the absence of long-range magnetic order. However, a broad hump in the specific heat at 1.6 K suggests short-range correlations. Neutron diffraction at low temperatures confirms the presence of three-dimensional antiferromagnetic correlations, manifested as diffuse magnetic scattering with a correlation length ξ=24.66Å and magnetic propagation vectors k=(121212) and (00.6250) at 20 mK.

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